Observation of three weakly bound valence states of I2.

Observation of three weakly bound valence states of I2. Research Abstract Details 

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Observation of three weakly bound valence states of I2. Abstract Text:

Trevor Ridley,Kenneth P Lawley,Robert J Donovan,Trevor Ridley,Kenneth P Lawley,Robert J Donovan,

Structured emission in the gas phase to two weakly bound valence states that correlate with the third dissociation limit, I*(2P1/2)+I*(2P1/2), designated as (bb), from two third tier ion-pair states of I2 correlating with I-(1S0)+I+(1D2), the 1g(1D2), and F'0u+(1D2) states, has been observed for the first time. The 1u(bb) state is shown to be bound by 377+/-2 cm(-1) and molecular constants have been determined. Vibrational structure in the 0g+(bb) state could not be resolved but the spectrum is consistent with the state being bound by 435 cm(-1). The relative integrated intensities of the emissions from both ion-pair states to various valence states have also been measured, and some aspects are rationalized in terms of the electronic configurations of the upper and lower states. Bound levels of a previously uncharacterized 1g(ab) valence state have also been observed in emission from the gamma1u(3P2) ion-pair state. The lower state is shown to be bound by 270+/-2 cm(-1) and molecular constants have been determined.

Observation of three weakly bound valence states of I2. Publishing Authors By Initials

T Ridley,KP Lawley,RJ Donovan,T Ridley,KP Lawley,RJ Donovan,

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Observation of three weakly bound valence states of I2. Journal Published:

PUBLICATION TYPE: Journal Article

Journal: The Journal of chemical physics

VOLUME: 127

Page Numbers: 154306

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ISSN: 0021-9606

DAY: 21

MONTH: Oct

YEAR: 2007

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LANGUAGE: eng

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AFFILIATION: School of Chemistry, The University of Edinburgh, West Mains Road, Edinburgh EH9 3JJ, Scotland, United Kingdom. t.ridley@ed.ac.uk

Country: United States

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MEDLINETA: J Chem Phys

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