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Nonaffine deformation of inherent structure as a static signature of cooperativity in supercooled liquids.

Nonaffine deformation of inherent structure as a static signature of cooperativity in supercooled liquids. Research Abstract Details 

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  • Nonaffine deformation of inherent structure as a static signature of cooperativity in supercooled liquids. Abstract Text:

    We unveil the existence of nonaffinely rearranging regions in the inherent structures (IS) of supercooled liquids by numerical simulations of model glass formers subject to static shear deformations combined with local energy minimizations. In the liquid state IS, we find a broad distribution of large rearrangements which are correlated only over small distances. At low temperatures, the onset of the cooperative dynamics corresponds to much smaller displacements correlated over larger distances. This finding indicates the presence of nonaffinely rearranging domains of relevant size in the IS deformation, which can be seen as the static counterpart of the cooperatively rearranging regions in the dynamics. This idea provides new insight into possible structural signatures of slow cooperative dynamics of supercooled liquids and supports the connections with elastic heterogeneities found in amorphous solids.

    Nonaffine deformation of inherent structure as a static signature of cooperativity in supercooled liquids. Publishing Authors By Initials

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    Nonaffine deformation of inherent structure as a static signature of cooperativity in supercooled liquids. Journal Published:

    PUBLICATION TYPE: Journal Article

    Journal: Physical review letters

    VOLUME: 101

    Page Numbers: 095501

    Journal Abbreviation:

    ISSN: 0031-9007

    DAY: 25

    MONTH: 08

    YEAR: 2008

    Nonaffine deformation of inherent structure as a static signature of cooperativity in supercooled liquids. Information

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    LANGUAGE: eng

    NlmUniqueID: 401141

    Nonaffine deformation of inherent structure as a static signature of cooperativity in supercooled liquids. Keywords Mesh Terms:

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    Grant and Affiliation Information for Nonaffine deformation of inherent structure as a static signature of cooperativity in supercooled liquids.

    AFFILIATION: ETH Zürich, Polymer Physics, CH-8093 Zürich, Switzerland.

    Country: United States

    United States Research PublicationUnited States Research Publication

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    MEDLINETA: Phys Rev Lett

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